Carrier multiplication in germanium nanocrystals

Carrier multiplication is demonstrated in a solid-state dispersion of germanium nanocrystals in a silicon-dioxide matrix. This is performed by comparing ultrafast photo-induced absorption transients at different pump photon energies below and above the threshold energy for this process. The average...

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Bibliographic Details
Main Author: Saeed, Saba (author)
Other Authors: de Weerd, Chris (author), Stallinga, Peter (author), Spoor, Frank C. M. (author), Houtepen, Arjan J. (author), Siebbeles, Laurens D. A. (author), Gregorkiewicz, Tom (author)
Format: article
Language:eng
Published: 2018
Subjects:
Online Access:http://hdl.handle.net/10400.1/11277
Country:Portugal
Oai:oai:sapientia.ualg.pt:10400.1/11277
Description
Summary:Carrier multiplication is demonstrated in a solid-state dispersion of germanium nanocrystals in a silicon-dioxide matrix. This is performed by comparing ultrafast photo-induced absorption transients at different pump photon energies below and above the threshold energy for this process. The average germanium nanocrystal size is approximately 5-6 nm, as inferred from photoluminescence and Raman spectra. A carrier multiplication efficiency of approximately 190% is measured for photo-excitation at 2.8 times the optical bandgap of germanium nanocrystals, deduced from their photoluminescence spectra.